Architected materials (or mechanical metamaterials) across length scales—from nanometers to centimeters—have enabled previously unachievable mechanical properties through a variety of 3D material morphologies. Significant advances in our understanding of these materials have thus pointed to structure-property relations that lead to unique macroscopic mechanical properties. Despite this progress, several hurdles have precluded widespread application of these materials to solve engineering challenges. First, clear routes to scalably design and fabricate these architected materials have remained elusive; with most designs reported to date targeting high stiffness but low deformability. Second, since most of the studies to date have characterized architected materials under quasi-static deformation, their dynamic-property regime remains to be fully characterized and understood—essential to a variety of envisioned applications. In this talk, we present efforts towards addressing these long-standing challenges, specifically by proposing routes for designing architected materials with extreme compliance and by presenting two types of high-throughput characterization methods that enable exploration of architected materials under dynamic conditions. We discuss efforts implementing and understanding compliant architected materials by proposing metamaterial design paradigms inspired by polymer-network architectures. We also present efforts performing non-contact characterization of materials through laser-induced vibrational signatures, providing a new route to uncover dynamic elastic responses of materials and unparalleled throughput rates. Lastly, we discuss efforts characterizing architected materials under extreme dynamic conditions through use of microparticle impact experiments at the microscale, shedding light on energy dissipation mechanisms that emerge from the use of 3D microstructure.